The high fps alone could definitely account for the crashing, or it could be causing your hardware to overheat and your system to crash the game in response. Either way, running at 60 fps should help a lot. If you have an Nvidia graphics card, you can enable vertical sync through the built-in Control Panel, although this doesn't always work (and only ever works in fullscreen mode). This guide has good screenshots of the CP, under the first spoiler:
https://forums.thesims.com/en_US/discussion/comment/16540301/#Comment_16540301
If CP doesn't work, you can download Nvidia Inspector (free) and manually limit fps. Or, if the driver for your graphics card is new enough, you'll have the option to set a max framerate in the Control Panel, which works in either fullscreen or windowed mode. (CP > Manage 3D Settings > Max Frame Rate; set to On and limit fps to 60.)
If you have an AMD graphics card, you can try the built-in Crimson software: create a profile for Sims 3 and have a look around. (I don't know exactly what all the options look like in the new software.) If that doesn't work, you can download RivaTuner Statistics Server (also free) and manually cap fps at 60. Unlike the others, RTSS does need to be running while you play, so be sure to minimize it rather than Xing it out. You can also use it with an Nvidia card if you want.
In any case, to create the profile for Sims 3, you'll need to use TS3.exe for an Origin install, or TS3W.exe (with the W) for a disc or Steam install. If one tool doesn't work, just move on to the next one.