Thanks so much for your continued help with this!
The results I got are below:
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Thanks :) As you can see from the file path the Tray folder is still in iCloud. You need to free up space on your internal drive and disable iCloud Drive syncing your Documents folder so the Electronic Arts > The Sims 4 folder containing all your user data is in the local Documents folder. I've merged your thread into the master iCloud thread. More info in the opening post.
