@IAmTaylorAnn Origin settings only cover where the game's program files go. If you want to move the Sims 4 user folder, you'll need to set up a symbolic link. Here's a guide:
https://crinrict.com/blog/2020/02/moving-windows-documents-folder-to-external-drive-via-symbolic-link.html
Please make a backup copy of the Sims 4 user folder before you try this, just in case something goes wrong.
And keep in mind that having the user folder on an SD card can increase loading times, perhaps by a significant amount if you use a lot of custom content.
